SYNTHESIS AND MAGNETIC PROPERTIES OF Co1−xCuxCr2S4 (x = 0–0.6) SOLID SOLUTIONS

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Resumo

Solid solutions Co1−xCuxCr2S4 (x = 0–0.6) between ferrimagnet CoCr2S4 (Tc = 222 K) and ferromagnet CuCr2S4 (Tc = 367 K) were synthesized by the solid-phase method. Magnetic properties were investigated by the dynamic method in the temperature range of 5–300 K at different frequencies (100, 1000, 5000 and 10000 Hz) of an alternating magnetic field with an amplitude of 1 Oe. The temperatures and nature of magnetic phase transitions in the system were determined. Substitution of Co by Cu from x = 0 to x = 0.6 increases the magnetic ordering temperature from 222 K to 287 K, respectively. A transition to a frustrated state of the spin glass type was detected in the sample with x = 0.05.

Sobre autores

E. Busheva

N. S. Kurnakov Institute of General and Inorganic Chemistry, Russian Academy of Sciences

Email: busheva@igic.ras.ru
Moscow, Russia

M. Suanov

N. S. Kurnakov Institute of General and Inorganic Chemistry, Russian Academy of Sciences

Email: busheva@igic.ras.ru
Moscow, Russia

G. Shabunina

N. S. Kurnakov Institute of General and Inorganic Chemistry, Russian Academy of Sciences

Email: busheva@igic.ras.ru
Moscow, Russia

P. Vasilev

N. S. Kurnakov Institute of General and Inorganic Chemistry, Russian Academy of Sciences

Autor responsável pela correspondência
Email: busheva@igic.ras.ru
Moscow, Russia

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